Facilities

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The first tests were the HEVA series conducted between 1983 and 1989 where, with maximum temperatures restricted to 2100K, the main objective was to generate information on release of volatile FPs from UO2 fuel. Between 1989 and 1996, the tests VERCORS 1 to 6 were conducted with an improved apparatus and fuel temperatures up to 2600K, i.e., higher than those in HEVA so as to expand assessment of release to lower volatility FPs and begin to address issues of UO2 fuel degradation. The apparatus also allowed, to a limited extent, investigation of FP transport.



Between 1996 and 2002, the test series VERCORS HT and RT were performed where the main intention was to improve the database with respect to transport aspects and FP release during later accident phases, i.e., encompassing highly-degraded fuel states (debris, liquefaction). The effect of other parameters on FP release was also studied, notably the influence of high fuel burn-up (up to 70GWd/tU) and mixed-oxide fuel (MOX). The particularity of the RT series was the simplification of the apparatus downstream of the crucible allowing better quantification of low-level releases. Eight RT tests were performed in a variety of atmospheres, namely pure hydrogen, steam-hydrogen mixtures and one test with a helium-air mixture. The particularity of the HT tests was that they included a well-characterized transport system downstream of the crucible allowing deposition and sampling measurements to be made. This series comprised three complementary tests covering the full range of H2-H2O atmospheres with and without the presence of control-rod elements (Ag-In-Cd-B) in order to assess their effect on FP retention.



All six VERCORS tests, most of the VERCORS RT tests and all three HT tests included low- power re-irradiation of the fuel sample in an experimental reactor for a week to re-create the short half-life FP inventory. This allowed the measurement of lower volatility FPs to be considerably enriched. Furthermore, all except three of these tests were conducted with an intermediate temperature plateau (1500K or 1800K) lasting one hour such that full oxidation of the cladding occurred and early sample liquefaction was precluded.



IRSN has for some time been using its computer codes to analyse the results of the VERCORS tests. These codes are the mechanistic release code MFPR [2,3], the simplified release code ELSA [4] (a module of the integral code ASTEC [5]) and the transport code SOPHAEROS [6] (also a module of ASTEC). Regarding the study of FP release, the focus of this work has been on VERCORS 4 and 5 as well as some of the RT tests. In particular, the detailed interpretation made possible with the MFPR code is shedding light on how the oxidation state of the fuel affects the FP chemistry modifying the different fuel phases. Most notably, it is currently thought that the FP Mo, often considered a main component of metallic inclusions during reactor operations, acts to a certain extent as an oxygen buffer (by forming MoO2) with respect to other FPs, i.e., playing a key regulatory role in the chemical forms of the FPs, especially Cs, and hence their volatility and release [7]. With respect to FP transport, the HT tests represent the major interest. Currently, full results of the HT1 test have been available for some time; those of HT3 have just recently been finalized while HT2 was performed in 2002 and results are still awaited. Hence, interpretation of the transport results is, as yet, preliminary [8]. In general terms, it is seen that the usual release categories of volatile, semi-volatile and low volatility FPs can be quite misleading during transport since behaviour can change radically as a function of the in-fuel and ex-fuel differences. One particular point of interest concerns the distinctive difference in behaviour between caesium and iodine where iodine seems to exhibit volatile behaviour whatever the conditions while Cs tends towards different levels of intermediate volatility depending on the reactive species present (molybdenum, boron, etc.). Another aspect being investigated is the conditions leading to significant deposition of so-called semi-volatile FPs (Ba, Mo, Ru, etc.) close to their point of release.

Facility is dismanteled, replaced by VERDON.

Since the core meltdown accident in the Three Mile Island reactor in 1979, a series of experimental safety research programmes has been conducted by a number of international research organisations, including the IRSN, which manages the European SARNET network. Simulation models have been developed to calculate the sequence of events in an accident of this type, evaluate its consequences and assess the efficacy of the various measures that can be implemented to limit its effects.



The PHEBUS FP research programme was launched in 1988 by the IRSN (under the former name IPSN – Institut de Protection et de Sûreté Nucléaire, Nuclear Protection and Safety Institute) in partnership with the European Commission and EDF. France collaborated in this programme with the United States, Canada, Japan, South Korea and Switzerland, and five experiments were conducted between 1993 and 2004, involving approximately 80 persons per year.



The main objective was to reduce the uncertainty in evaluating the release of radioactive products in the event of a core meltdown accident in a pressurised water reactor (PWR). To do this, “global” experiments were conducted, that is, experiments in which all the phenomena were represented, from melting of a fuel assembly to release of fission products and structural materials inside a simulated containment vessel, duplicating as closely as possible the conditions that would apply in an accident of this type. The programme had the simultaneous aim of developing and validating the simulation software used to calculate the progression of the accident. This research was to contribute to improving IRSN crisis management by optimising the activities and procedures that would be implemented in the event of a nuclear accident to protect the population and the environment.

Facility is dismanteled.

This programme is dedicated to studying iodine chemistry under thermal non equilibrium (impact of chemical kinetics) in the primary cooling system in the event of a core meltdown accident in a water reactor.

The CHIP programme follows two axes which respectivly aims to:

• Identify physico-chemical elements which may have a reaction with iodine during his transfert from core to containment structure (short transfert duration, fast cooling...) and also identify chemical species which influence presence of volatile iodine;
• Get kinetics datas of the main reactions.

So as to fulfill these objectives, the experimental programme uses more or less complex "phenomenolgy" lines in the form of experimental facilities and a "analytical" line.



The data collected will be used to validate the transport models for iodine in the primary cooling system, which are integrated in the ASTEC software. This software is developed by the DPAM to predict the different types of possible accidents and the related radioactive product releases.



The CHIP programme is run by IRSN/DPAM and is part of the International Source Term Programme co-funded by the CEA, EDF, IRSN, the European Commission, the US Nuclear Regulatory Commission (NRC), the Atomic Energy of Canada Limited (AECL), the Korea Institute of Nuclear Safety the Paul Scherrer Institute and SUEZ-Tractebel over the 2005-2012 period.

Facility is in operation.

This emission has an impact on the iodine chemistry (AgI) and on the behavior of aerosols in the reactor primary circuit and in the containment. The presence of control rod material influences the source term potentially present in a PWR containment and likely to in the atmosphere.


In a French 900 PWR the AIC material can make up as much as 2 tons.


The results of these experiments should help in establishing computer models on the AIC source term, part of the ESCADRE (later ASTEC) code system. They should also be used as an experimental input for the AIC injection into VERCORS fuel release experiments.

Facility is not operating.

Iodine is a fission product of major importance, because volatile species can be formed under severe nuclear reactor accident conditions, and may potentially be released into the environment, leading to significant radiological consequences. The CAIMAN programme was devoted to studying the radiochemistry of iodine in the reactor containment in case of a severe accident occurring in a Pressurised Water Reactor; this is a data base of prime importance for the validation of codes, namely IODE, which is a module of the integral ASTEC (Accident Source Term Evaluation Code) code, jointly developed by the IRSN and the GRS. These computations are generally used to predict the radiological consequences of such an accident. The experimental programme, which ran from 1996 to 2002, concerned eighteen experiments in a facility of intermediate scale (300 dm3), where labelled iodine, 131I, was used to perform -counting. The CAIMAN tests are here analysed, and the main experimental observations and trends are described. For each experiment, IODE computations were performed and compared with experimental results in order to assess the possible weak points of the present modelling and to identify key parameters. Broadly speaking, the gaseous concentrations predicted are quite consistent with the experimental ones; the remaining gaps have been identified.
Facility is not operating.

The purpose of the SISYPHE (Simulation du Système Phébus Enceinte) facility at Cadarache was to build a 1:1 replica of the Phébus FP experimental containment vessel, assisting the Phébus test interpretation, for all phenomena concerning thermal-hydraulics and fission product behaviour.



All systems of the Phébus FP containment vessel are reproduced, except radiation. Instrumentation improved as compared to Phébus, by special optical instruments.



The objective of the testing foreseen in this vessel was manifold:

• A: Thermal Hydraulics Studies: these tests are simulating phenomena like: condensation on condensers and walls, convection, humidity up to 100%, presence of hot/cold sump, steam condensation on aerosols, diffusiophoresis, and iodine affinity with water. B: Aerosol Behaviour Programme: multicomponent aerosols from POLYR generator, soluble or non-soluble. Study on wall deposits or electrophoresis.
• B: Iodine Programme: studying the presence of molecular gaseous iodine, transfer to surfaces, interactions with paint, re-emission from sump by radiolysis, iodine aerosol interaction, and interface with hydrogen.
• C: Mass Transfer Programme: effect of evaporating or non-evaporating sump on molecular iodine mass transfer (in preparation to FPT2 & FPT3). Oxygen is the simulant for iodine. Ultimate goal: mass-transfer model to predict MT coefficient for oxygen and hence for iodine.

Duration of the programme: post-FPT1, between 1995 and 2003.

Facility is dismanteled, part of Phébus.

This programme will help to better estimate the quantity of radioactive iodine released during a core meltdown accident taken into account when elaborating specific emergency plans. The programme results will also be used to better define the means and measures required to limit releases into the environment.



A study on ruthenium chemistry – another radiotoxic product – in the reactor containment under accidental conditions was conducted as part of the ISTP. About twenty tests were performed to assess the effect of irradiation on the volatilisation of ruthenium from the sump or deposits on painted containment surfaces. This study provided experimental data used to determine ruthenium quantities released into the environment in the event of an accident.



Various materials can be irradiated so as to determine the impact of the received dose on the variation in certain properties. This application could be used to study the ageing of polymers, greases and other compounds, which would help improve existing computer models and make it possible to make more informed decisions on the reactor life extension for example.

Facility is in operation.

In case of a hypothetical severe accident in a nuclear LWR (light water reactor), the high radiation fields reached in the reactor containment building due to the release of fission products from the reactor core could induce air radiolysis. The air radiolysis products could, in turn, oxidise gaseous molecular iodine into aerosol–borne iodine–oxygen–nitrogencompounds. Thereby, this reaction involves a change of iodine speciation and a decrease of iodine volatility in the reactor containment atmosphere. Kinetic data were produced within the PARIS project on the air radiolysis products formation and destruction, and on their reaction with molecular iodine, with the objective of developing and validating existing kinetic models.
The Program on Air Radiolysis and Iodine adsorption on Surfaces (PARIS) was therefore initiated in 2002 by IRSN in collaboration with AREVA NP, as part of the research programs performed to improve severe accident modelling and evaluation of subsequent fission product release into the environment with specific objective of measuring:
• the rate and amount of ARP production and destruction,
• rate and extent of radiolytic oxidation of molecular iodine into iodine oxides,
• the effect of the containment structural surfaces, namely decontamination coating (“paint”) and stainless steel, on radiolytic oxidation of I2,
• the effect of silver, representing silver-containing aerosol particles, on radiolytic oxidation of I2.
Important new features of the PARIS project were: (1) more realistic low iodine concentrations, (2) surface to volume ratios of paint, steel and silver surface area to containment volume ratio representative of LWR or PHEBUS containments, (3)higher steam fractions and (4) representative dose rates. The PARIS database, containing about 400 tests, was intended to provide data to develop and validate empirical models, and finally to derive a simplified model for ASTEC Code and other severe accident iodine codes.
Facility is not operating.

Mozart program to determine the air-oxidation kinetics of zirconium alloys at high temperature.



Because the current state of knowledge concerning the oxidation in air of zirconium alloy revealed unacceptably large gaps and large uncertainties, IRSN decided to launch the Mozart experimental program to supplement the databases and help to better understand and better model the mechanisms involved.



The temperature range studied was restricted to 600-1200°C, because beyond this temperature range, oxidation becomes catastrophic and precise knowledge of the phenomenon is not required. Different types of alloy (Zircaloy-4, M5TM and Zirlo) in different initial states (virgin, pre-oxidized, pre-hydrided to simulate the initial state of corroded cladding in the reactor) were studied. In these tests, synthetic air was used as the oxidizing medium, and the increased weight gain of the cladding due to oxidation was continuously recorded using a thermobalance.



For initially virgin cladding in the temperature range 800-1000°C, the experimental data revealed two kinetic regimes during oxidation at a given temperature. During the first phase, corresponding to the formation of a dense protective oxide on the initially bare metal, the oxidation rate falls, approximately following a parabolic function. After the cracking of this dense layer ('breakaway'), the second phase is characterized by a faster oxidation rate, which either remains constant or increases over time. The presence of nitrogen plays an important role in the degradation of the cladding in this accelerated regime, because a self-sustaining nitriding/oxidation mechanism generates the formation of a porous, non-protective oxide and causes creep in the cladding. Above 1000°C, the kinetic regime remains parabolic, and therefore rather slow, provided that there is sufficient oxygen in the oxidizing medium. Otherwise, nitrogen becomes preponderant in the oxidizing medium, and can then diffuse in the cladding and cause nitriding. The pre-oxidation layer can either have a protective effect or quite the opposite: an accelerating effect, according to the pre-oxide thickness and the temperature domain and the alloy concerned.



Based on these results, a new model for the oxidation of Zircaloy by air was incorporated in the Astec computational software package developed by IRSN to evaluate the consequences of a core meltdown accident.

Facility is not operating.

Characterisation methods:

Gaseous releases are continuously measured by a mass spectrometer connected to the furnace outlet. After each test, the different samples are subject to metallographic examination to determine the degradation mechanism : interactions between materials, formation and liquefaction of mixtures, and formation of oxide layers. These examinations are performed with an electron microprobe. As part of tests conducted in the Intermezzo furnace, non-destructive examinations (radiography and tomography) are also performed on control rod sections to characterise their state of degradation.

Facility is not operating.

SOURCE TERM is an international research programme carried out by IRSN and CEA (Commissariat à l’Energie Atomique) with the support of Electricité de France, the European Commission, the US Nuclear Regulatory Commission (US), GDF/ SUEZ/ Tractebel (Belgium), Atomic Energy Canada Limited (Canada), the Paul Scherrer Institute (Switzerland) and the Korea Institute of Nuclear Safety (representing a South Korean consortium).

This programme has a budget of about €30 million over 5 years to investigate four different experimental topics:

1. Studying iodine chemistry.
2. Degradation of boron carbide (B4C) control rods.
3. Consequences of fuel rod heating in air.
4. Fission product releases from irradiated fuel at high temperature.

Facility is closed.

Facility is not operating.

HEVA programme started a series of fission-product release experiments, which have been continued with the VERCORS programme. HEVA and the three VERCORS (RT and HT) series represent a total of 28 tests. The results of all these experiments (carried out by CEA with the support of IRSN and EDF) and their interpretation (by IRSN) have made a considerable contribution to the overall knowledge of fission-product release in severe-accident conditions.
Under eight HEVA tests, conducted between 1983 and 1989 where, maximum temperatures were restricted to 2100K. The main objective was to generate information on release of volatile FPs from UO2 fuel. Between 1989 and 1996, the tests VERCORS 1 to 6 were conducted with an improved apparatus and fuel temperatures up to 2600K, so as to expand assessment of release to lower volatility FPs and begin to address issues of UO2 fuel degradation.
Facility is dismanteled.